Please use this identifier to cite or link to this item: https://hdl.handle.net/11147/11587
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dc.contributor.authorCalcabrini, Mariano-
dc.contributor.authorGenç, Aziz-
dc.contributor.authorLiu, Yu-
dc.contributor.authorKleinhanns, Tobias-
dc.contributor.authorLee, Seungho-
dc.contributor.authorDirin, Dmitry N.-
dc.contributor.authorAkkerman, Quinten A.-
dc.date.accessioned2021-11-06T09:54:42Z-
dc.date.available2021-11-06T09:54:42Z-
dc.date.issued2021-
dc.identifier.issn2380-8195-
dc.identifier.urihttps://doi.org/10.1021/acsenergylett.0c02448-
dc.identifier.urihttps://hdl.handle.net/11147/11587-
dc.description.abstractCesium lead halides have intrinsically unstable crystal lattices and easily transform within perovskite and nonperovskite structures. In this work, we explore the conversion of the perovskite CsPbBr3 into Cs4PbBr6 in the presence of PbS at 450 degrees C to produce doped nanocrystal-based composites with embedded Cs4PbBr6 nanoprecipitates. We show that PbBr2 is extracted from CsPbBr3 and diffuses into the PbS lattice with a consequent increase in the concentration of free charge carriers. This new doping strategy enables the adjustment of the density of charge carriers between 10(19) and 10(20) cm(-3), and it may serve as a general strategy for doping other nanocrystal-based semiconductors.en_US
dc.description.sponsorshipEuropean Union's Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie GrantSKA South Africa [665385]; Generalitat de CatalunyaGeneralitat de CatalunyaGeneral Electric [2017 SGR 327]; Severo Ochoa program from Spanish MINECO [SEV-2017-0706]; CERCA Programme/Generalitat de Catalunya; European Union's Horizon 2020 research and innovation programme [823717]; European Research Council under the Horizon 2020 Framework Program (ERC Consolidator Grant SCALEHALO Grant) [819740]; FET-OPEN project [862656]en_US
dc.description.sponsorshipM.C. has received funding from the European Union's Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie Grant Agreement No. 665385. ICN2 acknowledges funding from Generalitat de Catalunya 2017 SGR 327. ICN2 is supported by the Severo Ochoa program from Spanish MINECO (Grant No. SEV-2017-0706) and is funded by the CERCA Programme/Generalitat de Catalunya. This project has received funding from the European Union's Horizon 2020 research and innovation programme under grant agreement No 823717 -ESTEEM3. M.V.K. acknowledges the support by the European Research Council under the Horizon 2020 Framework Program (ERC Consolidator Grant SCALEHALO Grant Agreement No. 819740) and by FET-OPEN project no. 862656 (DROP-IT).en_US
dc.language.isoenen_US
dc.publisherAmerican Chemical Societyen_US
dc.relation.ispartofACS Energy Lettersen_US
dc.rightsinfo:eu-repo/semantics/openAccessen_US
dc.subjectSulfur compoundsen_US
dc.subjectHalide perovskitesen_US
dc.titleExploiting the lability of metal halide perovskites for doping semiconductor nanocompositesen_US
dc.typeArticleen_US
dc.authoridSemiconductor dopingen_US
dc.institutionauthorGenç, Aziz-
dc.departmentİzmir Institute of Technology. Materials Science and Engineeringen_US
dc.identifier.volume6en_US
dc.identifier.issue2en_US
dc.identifier.startpage581en_US
dc.identifier.endpage587en_US
dc.identifier.wosWOS:000619803400036en_US
dc.identifier.scopus2-s2.0-85100316480en_US
dc.relation.publicationcategoryMakale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanıen_US
dc.identifier.doi10.1021/acsenergylett.0c02448-
dc.identifier.pmid33614964en_US
dc.identifier.wosqualityQ1-
dc.identifier.scopusqualityQ1-
item.grantfulltextopen-
item.openairecristypehttp://purl.org/coar/resource_type/c_18cf-
item.cerifentitytypePublications-
item.openairetypeArticle-
item.languageiso639-1en-
item.fulltextWith Fulltext-
crisitem.author.dept03.09. Department of Materials Science and Engineering-
Appears in Collections:Materials Science and Engineering / Malzeme Bilimi ve Mühendisliği
PubMed İndeksli Yayınlar Koleksiyonu / PubMed Indexed Publications Collection
Scopus İndeksli Yayınlar Koleksiyonu / Scopus Indexed Publications Collection
WoS İndeksli Yayınlar Koleksiyonu / WoS Indexed Publications Collection
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